Electronic Squeezing of Pumped Phonons: Negative U and Transient Superconductivity
12.05.2017 at 09:00
Advances in light sources and time resolved spectroscopy have made it possible to excite specific atomic vibrations in solids and to observe the resulting changes in electronic properties. I argue that in narrow-band systems the dominant symmetry-allowed coupling between electron density and dipole active modes implies an electron density-dependent squeezing of the phonon state which provides an attractive contribution to the electron- electron interaction, independent of the sign of the bare electron-phonon coupling and with a magnitude proportional to the degree of laser-induced phonon excitation. Reasonable excitation amplitudes lead to non-negligible attractive interactions that may cause significant transient changes in electronic properties including superconductivity. The mechanism is generically applicable to a wide range of systems, offering a promising route to manipulating and controlling electronic phase behavior in novel materials.
A 450, Theresienstr. 37